J. Phys. Soc. Jpn. 83, 104701 (2014) [5 Pages]
FULL PAPERS
- Full text:
- PDF (eReader) / PDF (Download) (1234 kB)
Received May 9, 2014; Accepted July 28, 2014; Published September 3, 2014
We can directly investigate the ground state in magnetization-plateau fields (plateau ground state) by neutron diffraction measurements. We performed neutron diffraction measurements on the spin-5/2 trimer substance SrMn3P4O14 in magnetization-plateau fields. The integrated intensities of magnetic reflections calculated using an expectation value of each spin in a plateau ground state of an isolated-trimer model are in agreement with those obtained experimentally in the magnetization-plateau fields. We succeeded in the direct observation of a plateau ground state in SrMn3P4O14.
©2014 The Physical Society of Japan
References
- (1 ) Strictly speaking, we cannot see a ground state itself at finite temperatures because of the thermal mixing of excited states. However, the influence of excited states is negligible in magnetization-plateau fields because the presence of an energy gap. Google Scholar
- 2 K. Hida, J. Phys. Soc. Jpn. 63, 2359 (1994). 10.1143/JPSJ.63.2359 Link, Google Scholar
- 3 M. Oshikawa, M. Yamanaka, and I. Affleck, Phys. Rev. Lett. 78, 1984 (1997). 10.1103/PhysRevLett.78.1984 Crossref, Google Scholar
- 4 K. Katsumata, H. Hori, T. Takeuchi, M. Date, A. Yamagishi, and J. P. Renard, Phys. Rev. Lett. 63, 86 (1989). 10.1103/PhysRevLett.63.86 Crossref, Google Scholar
- 5 Y. Ajiro, T. Goto, H. Kikuchi, T. Sakakibara, and T. Inami, Phys. Rev. Lett. 63, 1424 (1989). 10.1103/PhysRevLett.63.1424 Crossref, Google Scholar
- 6 M. Hase, I. Terasaki, K. Uchinokura, M. Tokunaga, N. Miura, and H. Obara, Phys. Rev. B 48, 9616 (1993). 10.1103/PhysRevB.48.9616 Crossref, Google Scholar
- 7 H. Kageyama, K. Yoshimura, R. Stern, N. V. Mushnikov, K. Onizuka, M. Kato, K. Kosuge, C. P. Slichter, T. Goto, and Y. Ueda, Phys. Rev. Lett. 82, 3168 (1999). 10.1103/PhysRevLett.82.3168 Crossref, Google Scholar
- 8 J. P. Renard, M. Verdaguer, L. P. Regnault, W. A. C. Erkelens, J. Rossatmignod, and W. G. Stirling, Europhys. Lett. 3, 945 (1987). 10.1209/0295-5075/3/8/013 Crossref, Google Scholar
- 9 M. Hase, I. Terasaki, and K. Uchinokura, Phys. Rev. Lett. 70, 3651 (1993). 10.1103/PhysRevLett.70.3651 Crossref, Google Scholar
- 10 M. Hase, I. Terasaki, Y. Sasago, K. Uchinokura, and H. Obara, Phys. Rev. Lett. 71, 4059 (1993). 10.1103/PhysRevLett.71.4059 Crossref, Google Scholar
- 11 Ch. Rüegg, M. Oettli, J. Schefer, O. Zaharko, A. Furrer, H. Tanaka, K. W. Kramer, H. U. Gudel, P. Vorderwisch, K. Habicht, T. Polinski, and M. Meissner, Phys. Rev. Lett. 93, 037207 (2004). 10.1103/PhysRevLett.93.037207 Crossref, Google Scholar
- 12 M. Hase, M. Matsuda, K. Kakurai, K. Ozawa, H. Kitazawa, N. Tsujii, A. Dönni, M. Kohno, and X. Hu, Phys. Rev. B 76, 064431 (2007). 10.1103/PhysRevB.76.064431 Crossref, Google Scholar
- 13 M. Hase, M. Matsuda, K. Kaneko, N. Metoki, K. Kakurai, T. Yang, R. Cong, J. Lin, K. Ozawa, and H. Kitazawa, Phys. Rev. B 84, 214402 (2011). 10.1103/PhysRevB.84.214402 Crossref, Google Scholar
- (14 ) As described herein, it is defined that the sign of a magnetic moment is positive (negative) when the sign of a spin value is positive (negative). Google Scholar
- 15 T. Yang, Y. Zhang, S. Yang, G. Li, M. Xiong, F. Liao, and J. Lin, Inorg. Chem. 47, 2562 (2008). 10.1021/ic702346e Crossref, Google Scholar
- 16 M. Hase, T. Yang, R. Cong, J. Lin, A. Matsuo, K. Kindo, K. Ozawa, and H. Kitazawa, Phys. Rev. B 80, 054402 (2009). 10.1103/PhysRevB.80.054402 Crossref, Google Scholar
- 17 M. Hase, V. Yu. Pomjakushin, L. Keller, A. Dönni, O. Sakai, T. Yang, R. Cong, J. Lin, K. Ozawa, and H. Kitazawa, Phys. Rev. B 84, 184435 (2011). 10.1103/PhysRevB.84.184435 Crossref, Google Scholar
- 18 P. Fischer, G. Frey, M. Koch, M. Koennecke, V. Pomjakushin, J. Schefer, R. Thut, N. Schlumpf, R. Buerge, U. Greuter, S. Bondt, and E. Berruyer, Physica B 276–278, 146 (2000); 10.1016/S0921-4526(99)01399-X Crossref;, Google ScholarWeb [http://sinq.web.psi.ch/hrpt]. Google Scholar
- 19 J. Rodríguez-Carvajal, Physica B 192, 55 (1993); 10.1016/0921-4526(93)90108-I Crossref;, Google ScholarWeb [http://www.ill.eu/sites/fullprof/]. Google Scholar
- 20 A. Rauch and W. Waschkowski, in Neutron Data Booklet, ed. A.-J. Dianoux and G. Lander (Institut Laue-Langevin, Grenoble, 2003) Chap. 1.1. Google Scholar
- 21 S. W. Lovesey, Theory of Neutron Scattering from Condensed Matter (Oxford University Press, Oxford, U.K., 1984) Vol. 2. Google Scholar
- 22 V. Yu. Pomjakushin, A. Furrer, D. V. Sheptyakov, E. V. Pomjakushina, and K. Conder, Phys. Rev. B 76, 174433 (2007). 10.1103/PhysRevB.76.174433 Crossref, Google Scholar
- 23 V. Pomjakushin, arXiv:1404.1683. Google Scholar
- 24 A. Podlesnyak, V. Pomjakushin, E. Pomjakushina, K. Conder, and A. Furrer, Phys. Rev. B 76, 064420 (2007). 10.1103/PhysRevB.76.064420 Crossref, Google Scholar